Controlling single diamond NV color center photoluminescence spectrum with a Fabry-Perot microcavity

We present both theoretical and experimental results on fluorescence of single defect centers in diamond nanocrystals embedded in a planar dielectric microcavity. From a theoretical point of view, we show that the overall fluorescence collection efficiency using moderate numerical aperture microscope objective can be enhanced by using a low quality factor microcavity. This could be used in particular for low temperature applications where the numerical aperture of collection microscope objectives is limited due to the experimental constraints. We experimentally investigate the control of the fluorescence spectrum of the emitted light from a single center. We show the simultaneous narrowing of the room temperature broadband emission spectrum and the increase of the fluorescence spectral density.Comment: 22 pages, 10 figure

Narrow-band single-photon emission in the near infrared for quantum key distribution

We report on the observation of single colour centers in natural diamond samples emitting in the near infrared region when optically excited. Photoluminescence of these single emitters have several striking features, such as a narrow-band fully polarized emission (FWHM 2 nm) around 780 nm, a short excited-state lifetime of about 2 ns, and perfect photostability at room temperature under our excitation conditions. We present a detailed study of their photophysical properties. Development of a triggered single-photon source relying on this single colour centre is discussed in the prospect of its application to quantum key distribution.Comment: 9 page

Wheeler's delayed-choice thought experiment: Experimental realization and theoretical analysis

Wheeler has strikingly illustrated the wave-particle duality by the delayed-choice thought experiment, in which the configuration of a 2-path interferometer is chosen after a single-photon light-pulsed has entered it. We present a quantitative theoretical analysis of an experimental realization of Wheeler's proposal

Experimental realization of Wheeler's delayed-choice GedankenExperiment

The quantum "mystery which cannot go away" (in Feynman's words) of wave-particle duality is illustrated in a striking way by Wheeler's delayed-choice GedankenExperiment. In this experiment, the configuration of a two-path interferometer is chosen after a single-photon pulse has entered it : either the interferometer is \textit{closed} (\textit{i.e.} the two paths are recombined) and the interference is observed, or the interferometer remains \textit{open} and the path followed by the photon is measured. We report an almost ideal realization of that GedankenExperiment, where the light pulses are true single photons, allowing unambiguous which-way measurements, and the interferometer, which has two spatially separated paths, produces high visibility interference. The choice between measuring either the 'open' or 'closed' configuration is made by a quantum random number generator, and is space-like separated -- in the relativistic sense -- from the entering of the photon into the interferometer. Measurements in the closed configuration show interference with a visibility of 94%, while measurements in the open configuration allow us to determine the followed path with an error probability lower than 1%

Balanced homodyne detection in second-harmonic generation microscopy

We demonstrate the association of two-photon nonlinear microscopy with balanced homodyne detection for investigating second harmonic radiation properties at nanoscale dimensions. Variation of the relative phase between second-harmonic and fundamental beams is retrieved, as a function of the absolute orientation of the nonlinear emitters. Sensitivity down to approximately 3.2 photon/s in the spatio-temporal mode of the local oscillator is obtained. This value is high enough to efficiently detect the coherent second-harmonic emission from a single KTiOPO4 crystal of sub-wavelength size.Comment: 9 pages to appear in Applied Physics Letter

Comparison of the photoluminescence properties of semiconductor quantum dots and non-blinking diamond nanoparticles. Observation of the diffusion of diamond nanoparticles in living cells

Long-term observations of photoluminescence at the single-molecule level were until recently very diffcult, due to the photobleaching of organic ?uorophore molecules. Although inorganic semiconductor nanocrystals can overcome this diffculty showing very low photobleaching yield, they suffer from photoblinking. A new marker has been recently introduced, relying on diamond nanoparticles containing photoluminescent color centers. In this work we compare the photoluminescence of single quantum dots (QDs) to the one of nanodiamonds containing a single-color center. Contrary to other markers, photoluminescent nanodiamonds present a perfect photostability and no photoblinking. At saturation of their excitation, nanodiamonds photoluminescence intensity is only three times smaller than the one of QDs. Moreover, the bright and stable photoluminescence of nanodiamonds allows wide field observations of single nanoparticles motion. We demonstrate the possibility of recording the tra jectory of such single particle in culture cells

Magnetometry with nitrogen-vacancy ensembles in diamond based on infrared absorption in a doubly resonant optical cavity

We propose to use an optical cavity to enhance the sensitivity of magnetometers relying on the detection of the spin state of high-density nitrogen-vacancy ensembles in diamond using infrared optical absorption. The role of the cavity is to obtain a contrast in the absorption-detected magnetic resonance approaching unity at room temperature. We project an increase in the photon shot-noise limited sensitivity of two orders of magnitude in comparison with a single-pass approach. Optical losses can limit the enhancement to one order of magnitude which could still enable room temperature operation. Finally, the optical cavity also allows to use smaller pumping power when it is designed to be resonant at both the pump and the signal wavelength

Two-photon real-time device for single-particle holographic tracking (red shot)

Three-dimension real-time tracking of single emitters is an emerging tool for assessment of biological behavior as intraneuronal transport, for which spatiotemporal resolution is crucial to understand the microscopic interactions between molecular motors. We report the use of second harmonic signal from nonlinear nanoparticles to localize them in a super-localization regime, down to 15 nm precision, and at high refreshing rates, up to 1.1 kHz, allowing us to track the particles in real-time. Holograms dynamically displayed on a digital micro-mirror device are used to steer the excitation laser focus in 3D around the particle on a specific pattern. The particle position is inferred from the collected intensities using a maximum likelihood approach. The holograms are also used to compensate for optical aberrations of the optical system. We report tracking of particles moving faster than 30 $\mu$m/s with an uncertainty on the localization around 40 nm. We have been able to track freely moving particles over tens of micrometers, and directional intracellular transport in neurites